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Produktbild: Inert Gases
Band 34

Inert Gases Potentials, Dynamics, and Energy Transfer in Doped Crystals

Aus der Reihe Springer Series in Chemical Physics

Fr. 137.00

inkl. gesetzl. MwSt., Versandkostenfrei

Beschreibung

Produktdetails

Einband

Taschenbuch

Erscheinungsdatum

22.12.2011

Herausgeber

M.L. Klein

Verlag

Springer Berlin

Seitenzahl

268

Maße (L/B/H)

23.5/15.5/1.6 cm

Gewicht

435 g

Auflage

Softcover reprint of the original 1st ed. 1984

Sprache

Englisch

ISBN

978-3-642-82223-0

Beschreibung

Produktdetails

Einband

Taschenbuch

Erscheinungsdatum

22.12.2011

Herausgeber

M.L. Klein

Verlag

Springer Berlin

Seitenzahl

268

Maße (L/B/H)

23.5/15.5/1.6 cm

Gewicht

435 g

Auflage

Softcover reprint of the original 1st ed. 1984

Sprache

Englisch

ISBN

978-3-642-82223-0

Herstelleradresse

Springer-Verlag KG
Sachsenplatz 4-6
1201 Wien
AT

Email: GPSR Kontakt

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  • Produktbild: Inert Gases
  • 1. Argon and Its Companions..- 1.1 Prologue: Inert, Rare or Noble?.- 1.2 Research with Inert Gases.- 1.3 Outline of the Present Book.- References.- 2. Interatomic Potentials for Rare-Gases: Pure and Mixed Interactions.- 2.1 Background.- 2.2 What Probes What?.- 2.2.1 Bulk Properties.- 2.2.2 Molecular-Beam Experiments.- 2.2.3 Spectroscopic Data.- 2.3 Review of Recent Research on Pure Interactions.- 2.3.1 Helium.- 2.3.2 Neon.- 2.3.3 Argon.- 2.3.4 Krypton.- 2.3.5 Xenon.- 2.4 Review of Recent Research on Unlike Interactions.- 2.4.1 Helium-Rare-Gas Systems (He-Ne, He-Ar, He-Kr and He-Xe).- 2.4.2 Neon-Rare-Gas Systems (Ne-Ar, Ne-Kr, Ne-Xe).- 2.4.3 Argon-Krypton, Argon-Xenon, Krypton-Xenon.- 2.5 Combining Rules.- 2.5.1 Berthelot-Lorentz Rules.- 2.5.2 Kohler Rules.- 2.5.3 Hudson-McCoubrey Rules.- 2.5.4 Fender-Halsey Rules.- 2.5.5 Sikora Rules.- 2.5.6 Hiza-Duncan Rules.- 2.5.7 Total Cross-Section Rules.- 2.6 Conclusions.- Appendix: 2.A Interatomic Potential Functions.- 2.B Interatomic Potential Parameters.- 2.C Predictions of Collisons Cross-Sections by Potentials.- References.- 3. Dynamics of Impure Rare-Gas Crystals.- 3.1 Background.- 3.2 Lattice Dynamics of Impure Crystals.- 3.2.1 Historical Review.- 3.2.2 Pure Crystals.- 3.2.3 An Isolated Impurity.- 3.2.4 Central Force-Constant Model.- 3.2.5 Far-Infrared Absorption.- 3.2.6 Mossbauer Effect.- 3.2.7 Heat Capacity.- 3.2.8 Neutron Scattering.- 3.3 Theoretical Studies.- 3.3.1 Application of the CFC Model.- a) Potentials.- b) Relaxation Effects.- c) Three-Body Forces.- d) Phonon Density of States.- 3.3.2 Computer Simulation.- 3.4 Experimental Studies.- 3.4.1 Rare Gases in RGS.- a) Argon Doped with Krypton.- b) Argon Doped with Neon.- c) Argon Doped with Helium.- d) Argon Doped with Xenon.- e) Krypton Doped with Argon.- f) Krypton Doped with Xenon.- 3.4.2 Molecules in RGS.- a) Homonuclear Diatomics.- b) Heteronuclear Diatomics.- c) RGS Doped with Methane.- 3.4.3 Matrix-Isolated Species.- a) Molecular Ions.- b) Molecules.- c) Atoms.- 3.5 Summary.- References.- 4. Spectroscopy of Vibrational and Rotational Levels of Diatomic Molecules in Rare-Gas Crystals.- 4.1 Background.- 4.2 Experimental Techniques and Results.- 4.2.1 Experimental Techniques.- a) Sample Preparation.- b) Spectroscopy (Conventional Versus Laser).- c) Saturation Spectroscopy or Hole Burning.- d) Time-Resolved Spectroscopy.- 4.2.2 Spectroscopic Studies of Ground Electronic State Molecules.- a) Vibrational Transitions.- b) Rotational Transitions.- c) Phonon Sidebands.- 4.2.3 Time-Resolved Experiments.- a) Infrared Spectroscopy.- b) Visible Spectroscopy.- 4.3 Intermolecular Interaction in Rare-Gas Crystals Containing Molecular Defects.- 4.3.1 Intermolecular Potential Between a Rare-Gas Atom and a Diatomic Molecule.- a) Atom-Atom Potential.- b) Multiparameter Potential Functions.- c) Ab Initio Potential Surfaces.- d) Charge Transfer and Hydrogen Bonding.- 4.3.2 The Interaction Hamiltonian.- a) Energy Levels.- b) Relaxation Processes.- 4.4 Perturbation of Energy Levels.- 4.4.1 Influence of a Diatomic Impurity on Lattice Energies.- a) Effect of Isotropic Terms.- b) Effect of Internal Molecular Motions.- c) Description of Lattice Vibrations Through Molecular Dynamics.- d) Phonon Sidebands in IR Spectra of the Guest Molecule.- 4.4.2 Perturbation of the Molecular Energy Levels.- a) Vibrational Matrix Shift.- b) Rotational Matrix Shift.- 4.5 Population Relaxation Processes.- 4.5.1 Radiative Relaxation.- 4.5.2 Vibrational Relaxation to Phonons.- 4.5.3 Vibration to Rotation Energy Transfer.- 4.5.4 Vibrational Energy Transfer.- a) Microscopic Processes Among Molecules in Rare-Gas Crystals.- b) Microscopic Probabilities for Vibrational Energy Transfer.- c) Macroscopic Kinetics for Vibrational Energy Transfer.- d) Comparison Between Theory and Experiment.- 4.5.5 Radiationless Rotational Relaxation.- a) The Direct Process.- b) Raman and Orbach Processes.- 4.6 Spectral Line Shapes and Dephasing Processes.- 4.6.1 Homogeneous Broadening: T1 and T2 Relaxation Processes.- 4.6.2 Vibrational Dephasing in Matrix-Isolated Molecules.- 4.6.3 Line Shape Function and Dephasing.- a) Isolated Vibrational Levels with a Large Spacing.- b) Additional Low-Energy Levels in the Molecule.- 4.6.4 Comparison Between Theory and Experiment.- 4.7 Concluding Remarks.- References.- Additional References with Titles.